I know that you can say something like "我跟她很熟“。 But can you make someone into a very 熟的人。 ex。 他们是我在大学最熟的人
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Yes you can. This is 100% correct.
This is from a Xiangsheng transcript by Guodegang using exactly that form, but in a slightly different context (talking about the audience that arrived). Some are familiar people, some are not: